Chemistry, Physics and Technology of Surface, 2021, 12 (4), 306-313.

Electron tunneling in the germanium/silicon heterostructure with germanium quantum dots: theory



DOI: https://doi.org/10.15407/hftp12.04.306

S. I. Pokutnyi, N. G. Shkoda

Abstract


It is shown that electron tunneling through a potential barrier that separates two quantum dots of germanium leads to the splitting of electron states localized over spherical interfaces (a quantum dot – a silicon matrix). The dependence of the splitting values of the electron levels on the parameters of the nanosystem (the radius a quantum dot germanium, as well as the distance D between the surfaces of the quantum dots) is obtained. It has been shown that the splitting of electron levels in the QD chain of germanium causes the appearance of a zone of localized electron states, which is located in the bandgap of silicon matrix. It has been found that the motion of a charge-transport exciton along a chain of quantum dots of germanium causes an increase in photoconductivity in the nanosystem.

It is shown that in the QD chain of germanium a zone of localized electron states arises, which is located in the bandgap of the silicon matrix. Such a zone of local electron states is caused by the splitting of electron levels in the QD chain of germanium. Moreover, the motion of an electron in the zone of localized electron states causes an increase in photoconductivity in the nanosystem. The effect of increasing photoconductivity can make a significant contribution in the process of converting the energy of the optical range in photosynthesizing nanosystems. It has been found that comparison of the splitting dependence of the exciton level Eех(а) at a certain radius a QD with the experimental value of the width of the zone of localized electron states arising in the QD chain of germanium, allows us to obtain the distances D between the QD surfaces.

It has been shown that by changing the parameters of Ge/Si heterostructures with germanium QDs (radius of a germanium QD, as well as the distance D between the surfaces of the QDs), it is possible to vary the positions and widths of the zones of localized electronic states. The latter circumstance opens up new possibilities in the use of such nanoheterostructures as new structural materials for the creation of new nano-optoelectronics and nano-photosynthesizing devices of the infrared range.


Keywords


splitting of electronic states; charge-transfer exciton; spherical interface; potential barrier; Coulomb interaction; quantum dots

Full Text:

PDF

References


Yakimov A.I., Dvurechensky A.V., Nikiforov A.I. Spatially Separated Excitons in Type II Heterostructures Ge/Si. JETP Lett. 2001. 73(6): 529. https://doi.org/10.1134/1.1387520

Yakimov A.I., Dvurechensky A.V., Nikiforov A.I. Spatially Separated Excitons in Heterostructures Ge/Si. JETP Lett. 2001. 119(3): 529. https://doi.org/10.1134/1.1387520

Pokutnyi S.I. Excitons based on spatially separated electrons and holes in Ge/Si heterostructures. Low Temp. Phys. 2016. 42(12): 1151. https://doi.org/10.1063/1.4973506

Pokutnyi S.I. Binding Energy of the Exciton of a Spatially Separated Electron and Hole in Quasi-Zero-Dimensional Semiconductor Nanosystems. Tech. Phys. Lett. 2013. 39(3): 233. https://doi.org/10.1134/S1063785013030139

Pokutnyi S.I. Exciton spectroscopy with spatially separated electron and hole in Ge/Si heterostructures germanium quantum dots. Low Temp. Phys. 2018. 44(8): 819. https://doi.org/10.1063/1.5049165

Pokutnyi S.I. Biexciton in nanoheterostructures of germanium quantum dots. Opt. Eng. 2017. 56(6): 067104. https://doi.org/10.1117/1.OE.56.6.067104

Pokutnyi S.I. Polarizability of germanium quantum dots with spatially separated electrons and holes in Ge/Si heterostructure. Philos. Mag. Lett. 2019. 99(10): 386. https://doi.org/10.1080/09500839.2019.1695165

Pokutnyi S.I. Polarizability of germanium quantum dots with spatially separated electrons and holes. The European Physical Journal Plus. 2020. 135(1): 74. https://doi.org/10.1140/epjp/s13360-019-00050-x

Smagina J., Dvurechensky A.V., Seleznev V.A. Optical properties of a chain of germanium quantum dots. Semiconductors. 2015. 49(8): 749. https://doi.org/10.1134/S1063782615060238

Landau L.D., Lifshitz E.M. Course of Theoretical Physics. In: Quantum Mechanics. V. 3. (New York: Pergamon Press, 1974). https://doi.org/10.1016/B978-0-08-017801-1.50007-5

Antonyuk B.P., Antonyuk V.P., Frolov A.A. Excitons with charge transfer in nanosystems. Opt. Commun. 2000. 174(4): 427. https://doi.org/10.1016/S0030-4018(99)00727-0




DOI: https://doi.org/10.15407/hftp12.04.306

Copyright (©) 2021 S. I. Pokutnyi, N. G. Shkoda

Creative Commons License
This work is licensed under a Creative Commons Attribution 4.0 International License.