ХІМІЯ, ФІЗИКА ТА ТЕХНОЛОГІЯ ПОВЕРХНІ

ISSN 2518-1238 (Online), ISSN 2079-1704 (Print)

У запропонованій роботі розглянуто водневосорбційні властивості систем магнієвих інтерметалідів зі складною кубічною структурою C15b як перспективних, надійних, реверсивних накопичувачів водню. Розглянуто теплові процеси. Запропоновано статистичну теорію для кубічної структури C15b складу MgRT₄H_x, де R = Ce, La, Nd, Pr, Y; T = Co, Ni; 0 ≤ x ≤ 6 при фазових переходах при гідруванні з урахуванням тиску. Встановлено концентраційну залежність максимальних значень параметра порядку та апріорних ймовірностей. Розраховано та розглянуто ізоплети та ізотерми розчинності водню та створено графічну концентраційну залежність температури впорядкування атомів водню в кристалах типу MgCeCo₄.

Розглянуто перехід порядок-безлад з урахуванням температури, а також вивчено процес абсорбції-десорбції водню структурою C15b. Виведено рівняння термодинамічної рівноваги із розрахунком вільної енергії, а також розглянуто графічну залежність значення параметра порядку від температури та тиску. Розглянуто температурну залежність розчинності водню у фазах α, β для кристала MgCeCo₄. Вивчено конфігураційну теплоємність кристала структури типу MgSnCu₄H_x при врахуванні температури та параметра порядку.

Побудовано графік водневої абсорбції-десорбції кристала MgCeCo₄H_x. Проведено порівняльний аналіз експериментальних та практичних результатів абсорбції-десорбції водню робочим тілом складу MgRT₄H_x.

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